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os.remove(path)

#!/usr/bin/python3

import os, sys

# List directory
print ("Directory is: %s" %os.listdir(os.getcwd()))

# Remove
os.remove("aa.txt")

# List directory after removal
print ("After removal: %s" %os.listdir(os.getcwd()))

Directory is:
[ 'a1.txt','aa.txt','resume.doc' ]
After removal: 
[ 'a1.txt','resume.doc' ]